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What is a Psychonaut?

source: Ayahuasca Visions, vision 45
Psychonautics goes hand-in-hand with the concept of introspection.
Introspection: self-observation and reporting conscious inner thoughts, desires and sensations.

Behaviorists claimed that introspection was unreliable and that the subject matter of scientific psychology should be strictly operationalized in an objective and measurable way. This then led psychology to focus on measurable behavior rather than consciousness or sensation.[1] Cognitive psychology accepts the use of the scientific method, but rejects introspection as a valid method of investigation for this reason.
Source:Wikipedia

What is a psychonaut?
A psychonaut (from the Greek ψυχοναύτης, meaning literally a sailor of the mind) is a person who uses trance technologies from any of the world's religions, modern psychology, meditation, and other assorted paradigms, to explore the psyche, their own consciousness, and potentially improve real performance of certain psychological tasks. The term is often associated with the use of hallucinogens or entheogens as guides, or means, to achieve inward spiritual experiences. This is quite distinct from religious use, or social and leisure use of drugs, although these can overlap.
According to Jonathan Ott, the word psychonaut was originally coined by the German author Ernst Jünger.

Concepts
Brain function
Psychonautics can be considered an attempt to generate a user's manual for the human brain. Unlike psychology, which is concerned with understanding other people, psychonauts are more concerned with understanding themselves, and the process of self exploration; accordingly, they engage in direct exploration of themselves and their own thought processes.
As such, psychonauts seek to experientially understand mental process and functioning and employ such knowledge in their activities. Key to this is auto-modification of brain wave frequencies, which can lead to quite distinct perceptual states; a detailed examination and understanding of one's own thought processes, habits, and beliefs is also sought. Hallucinatory states, drug-induced or otherwise, are seen as a form of subliminal symbolism or as a real but distinct reality; as with other processes of the mind, psychonauts seek to understand these. Psychological theories and concepts are also often taken into account, particularly those of Carl G. Jung and Abraham Maslow.
This is also ideally practically applied in bettering one's self through the knowledge of one's own thought processes; with this understanding and heightened perception of one's own internal dialogue, it is thought that one is more able to control their own ego, and detach themselves from what is seen as a herd mentality common to modern culture.

Mythical archetypes and concepts
Psychonauts, as described in the Tibetan Book of the Dead, place emphasis on various mythical archetypes and concepts, believing that these are useful to coming to understand one's own thought patterns and the nature of existence, reflecting realities and meanings that should be understood, rather than being irrelevant fantasy. As in shamanic practice, the Axis mundi is often employed, often overlayed with chakras and other relevant concepts of bodily function; the Kabbalist Tree of Life and its chakra-like sephirot is one notable example of this in mythology. The nature of karma is often explored in trying to understand one's own situation, actions, and relation to the outside world.

Metaphysics
Psychonauts are often interested in metaphysics, the branch of philosophy dealing with the ultimate nature of reality or existence; it is thought that in coming to some understanding of how the universe functions and the nature of existence, one would be better able to govern themselves accordingly and integrate their life experiences.
Source: Reference.com

Research papers and articles on the role of psychedelic substances in psychological and shamanic healing practices:
Documents for Serious Psychonauts

source: What is a Psychonaut?
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